I actually realized the column problem in COUNTROWS about five minutes after posting - thank you Chapter 7.
Shortly thereafter, I had a moment of clarity and defined separate measures for each bucket, subtracting the next "younger" to display only orders in the desired range. CALCULATE(COUNTROWS(OpenOrders), ('OpenOrders'[AgingDays]<7)-('OpenOrders'[AgingDays]<5))
The product:
[TABLE="width: 632"]
<COLGROUP><COL style="WIDTH: 69pt; mso-width-source: userset; mso-width-alt: 3364" width=92><COL style="WIDTH: 71pt; mso-width-source: userset; mso-width-alt: 3437" width=94><COL style="WIDTH: 54pt; mso-width-source: userset; mso-width-alt: 2633" span=2 width=72><COL style="WIDTH: 59pt; mso-width-source: userset; mso-width-alt: 2889" width=79><COL style="WIDTH: 65pt; mso-width-source: userset; mso-width-alt: 3145" span=5 width=86><TBODY>[TR]
[TD="width: 92"]
Row Labels[/TD]
[TD="width: 94"]Zero to 2 Days[/TD]
[TD="width: 72"]3 to 4 Days[/TD]
[TD="width: 72"]5 to 6 Days[/TD]
[TD="width: 79"]7 to 10 Days[/TD]
[TD="width: 86"]11 to 15 Days[/TD]
[TD="width: 86"]16 to 20 Days[/TD]
[TD="width: 86"]21 to 25 Days[/TD]
[TD="width: 86"]26 to 30 Days[/TD]
[TD="width: 86"]Over 30 Days[/TD]
[/TR]
[TR]
[TD="class: xl63, bgcolor: transparent"]1085[/TD]
[TD="bgcolor: transparent, align: right"]61[/TD]
[TD="bgcolor: transparent, align: right"]10[/TD]
[TD="bgcolor: transparent, align: right"]20[/TD]
[TD="bgcolor: transparent, align: right"]29[/TD]
[TD="bgcolor: transparent, align: right"]19[/TD]
[TD="bgcolor: transparent, align: right"]10[/TD]
[TD="bgcolor: transparent, align: right"]2[/TD]
[TD="bgcolor: transparent"][/TD]
[TD="bgcolor: transparent, align: right"]3[/TD]
[/TR]
[TR]
[TD="class: xl63, bgcolor: transparent"]1953[/TD]
[TD="bgcolor: transparent, align: right"]45[/TD]
[TD="bgcolor: transparent, align: right"]9[/TD]
[TD="bgcolor: transparent, align: right"]8[/TD]
[TD="bgcolor: transparent, align: right"]18[/TD]
[TD="bgcolor: transparent, align: right"]14[/TD]
[TD="bgcolor: transparent, align: right"]5[/TD]
[TD="bgcolor: transparent"][/TD]
[TD="bgcolor: transparent"][/TD]
[TD="bgcolor: transparent, align: right"]6[/TD]
[/TR]
[TR]
[TD="class: xl63"]Grand Total[/TD]
[TD="align: right"]106[/TD]
[TD="align: right"]19[/TD]
[TD="align: right"]28[/TD]
[TD="align: right"]47[/TD]
[TD="align: right"]33[/TD]
[TD="align: right"]15[/TD]
[TD="align: right"]2[/TD]
[TD][/TD]
[TD="align: right"]9[/TD]
[/TR]
</TBODY>[/TABLE]